RESEARCH PAPER
Sediment geochronology and spatio-temporal and vertical distributions of radionuclides in the Upper Bonny Estuary (South Nigeria)
 
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1
Department of Animal and Environmental Biology Faculty of Science, University of Port Harcourt, Port Harcourt, Nigeria
 
2
Centre National de L’Energie, des Sciences et des Techniques Nucléaires (CNESTEN), B.P. 1382, R.P. 10001, Rabat, Morocco
 
3
Centre for Marine Pollution Monitoring and Seafood Safety, University of Port Harcourt, Port Harcourt, Nigeria
 
 
Online publication date: 2014-10-01
 
 
Publication date: 2014-12-01
 
 
Geochronometria 2014;41(4):369-376
 
KEYWORDS
ABSTRACT
Surface deposits and sediment cores were collected from the Upper Bonny Estuary, located in Southwest Nigeria, and analyzed to determine spatio-temporal and vertical distributions of radio-nuclide activities expressed in Bq·kg−1 dry weight. The results of activities of naturally occurring radionuclides of 226Ra (15 ± 2–34 ± 3 Bq·kg−1), 228Ra (32 ± 5–48 ± 6 Bq·kg−1), 40K (264 ± 29–462 ± 36 Bq·kg−1) were found to be all within the range of typical values reported for coastal regions. Ratios of 226Ra to 228Ra suggested accretion for all samples with low sediment accumulation registered during rainy months. In addition, vertical distributions at the three sampling sites were also studied with the initial aim of establishing chronologies from the decay of excess 210Pb. In two cores, excess 210Pb, estimated by subtracting 226Ra from total 210Pb on a layer-by-layer basis, exhibit relatively constant activity with discrete minima and maxima. Therefore, these cores were excluded from radiometric dating. Only the third core could be dated by the constant rate of supply model, and 137Cs was utilized to validate the 210Pb chronology.
 
REFERENCES (27)
1.
Arogunjo AM, Hollriegl V, Giussani A, Leopold K, Gerstmann U, Veronese I and Oeh U, 2009. Uranium and thorium in soils, mineral sands, water and food samples in a tin mining area in Nigeria with elevated activity. Journal of Environmental Radioactivity 100(3): 232–240, DOI 10.1016/j.jenvrad.2008.12.004. http://dx.doi.org/10.1016/j.je....
 
2.
Agbalagba EO and Enoja RA, 2011. Evaluation of natural radioactivity in soil, sediment and water samples of Niger Delta (Biseni) flood plain lakes, Nigeria. Journal of Environmental Radioactivity 102(7): 667–671, DOI 10.1016/j.jenvrad.2011.03.002. http://dx.doi.org/10.1016/j.je....
 
3.
Alatise OO, Babalola IA and Olowofela JA, 2008. Distribution of some natural gamma-emitting radionuclides in the soils of the coastal areas of Nigeria. Journal of Environmental Radioactivity 99(11): 1746–1749, DOI 10.1016/j.jenvrad.2008.06.014. http://dx.doi.org/10.1016/j.je....
 
4.
Appleby PG and Oldfield F, 1992. Application of 210-lead to sedimen-tation studies. In: Ivanovich, M., Harmon, R.S. (Eds.), Uranium Series Disequilibrium: Appplications to Earth, Marine and Environmental Sciences, second ed. Oxford Science, Oxford, pp. 731–783.
 
5.
Appleby PG, 2008. Three decades of dating recent sediments by fallout radionuclides: a review. The Holocene 18(1): 83–93, DOI 10.1177/0959683607085598. http://dx.doi.org/10.1177/0959....
 
6.
Begy R, Timar-Gabor A, Somlai J and Cosma C, 2011. A sedimentation study of St. Ana Lake (Romania) applying the 210Pb and 137Cs dating methods. Geochronometria 38(2): 93–100, DOI 10.2478/s13386-011-0017-6. http://dx.doi.org/10.2478/s133....
 
7.
Brenner M, Claire L, Schelske CL and William FK, 2004. Inputs of dissolved and particulate 226Ra to lakes and implications for 210Pb dating recent sediments. Journal of Paleolimnology 32(1): 53–66, DOI 10.1023/B:JOPL.0000025281.54969.03. http://dx.doi.org/10.1023/B:JO....
 
8.
Dublin-Green CO, 1985. Some textural characteristics and organic matter contents of recent sediments in the Bonny Estuary, Niger Delta. Technical Paper N° 67. ISBN: 978-2345-069.
 
9.
Farai IP, Obed RI and Jibiri NN, 2006. Soil radioactivity and incidence of cancer in Nigeria. Journal of Environmental Radioactivity 90(1): 29–36, DOI 10.1016/j.jenvrad.2006.06.003. http://dx.doi.org/10.1016/j.je....
 
10.
Helz GR, Setlock GH, Cantillo AY, Moore WS, 1985. Processes con-trolling the regional distribution of 210Pb, 226Ra and anthropogenic zinc in estuarine sediments. Earth and Planetary Science Letters 76(1–2): 23–34, DOI 10.1016/0012-821X(85)90145-1. http://dx.doi.org/10.1016/0012....
 
11.
Imboden DM and Stiller M, 1982. Influence of radon diffusion on the 210Pb distribution in sediments. Journal of Geophysical Research: Oceans 87: 557–565, DOI 10.1029/JC087iC01p00557. http://dx.doi.org/10.1029/JC08....
 
12.
International Atomic Energy Agency, 2004. Sediment Distribution Coefficients and Concentration Factors for Biota in the Marine Environment. Technical Reports Series ISSN 0074-1914; no. 422.
 
13.
Inyang IR, Adeyemo AO and Ogamba EN, 2011. Impact of Waste Dump on Seasonal Fish Species Composition and Water Quality in the Upper Bonny Estuary. International Journal of Current Bio-logical and Medical Science 1(3): 90–94.
 
14.
Kirchner G, 2011. 210Pb as a tool for establishing sediment chronologies: examples of potentials and limitations of conventional dating models. Journal of Environmental Radioactivity 102(5): 490–494, DOI 10.1016/j.jenvrad.2010.11.010. http://dx.doi.org/10.1016/j.je....
 
15.
Kolb WA and Wojcik M, 1985. Enhanced radioactivity due to natural oil and gas production and related radiological problems. Science of the Total Environment 45: 77–84, DOI 10.1016/0048-9697(85)90206-2. http://dx.doi.org/10.1016/0048....
 
16.
Laissaoui A, Benmansour M, Ziad N, IbnMajah M, Abril JM and Mulsow S, 2008. Anthropogenic radionuclides in the water column and a sediment core from the Alboran Sea: Application to radiometric dating and reconstruction of historical water column radionuclide concentration. Journal of Paleolimnology 40(3): 823–833, DOI 10.1007/s10933-008-9201-y. http://dx.doi.org/10.1007/s109....
 
17.
Laissaoui A, Mas JL, Hurtado S, Ziad N, Villa M and Benmansour M, 2013. Radionuclide activities and metal concentrations in sediments of the Sebou Estuary, NW Morocco, following a flooding event. Environmental Monitoring and Assessment 185(6): 5019–5029, DOI 10.1007/s10661-012-2922-4. http://dx.doi.org/10.1007/s106....
 
18.
Leopold K and Gerstmann U, 2009. A comment on “Distribution of some natural gamma-emitting radionuclides in the soils of the coastal areas of Nigeria” by Alatise, O.O., Babalola, I.A. & Olowofela, J.A. Journal of Environmental radioactivity, 99 (2008) 1746–1749. Letter to Editor. Journal of Environmental radioactivity 100(7): 605, DOI 10.1016/j.jenvrad.2009.03.019. http://dx.doi.org/10.1016/j.je....
 
19.
Matthews KM, Kim CK and Martin P, 2007. Determination of 210Po in environmental materials: A review of analytical methodology. Applied Radiation and Isotopes 65(3): 267–279, DOI 10.1016/j.apradiso.2006.09.005. http://dx.doi.org/10.1016/j.ap....
 
20.
Noakes S, 2003. Postdisposal areal mapping of sediment chemistry at the Fort Pierce, Florida ODMDS. U.S. Environmental Protection Agency, Final Report.
 
21.
Pfitzner J, Brunskill G and Zagorskis I, 2004. 137Cs and excess 210Pb deposition patterns in estuarine and marine sediment in the central region of the Great Barrier Reef Lagoon, north-eastern Australia. Journal of Environmental Radioactivity 76(1–2): 81–102, DOI 10.1016/j.jenvrad.2004.03.020. http://dx.doi.org/10.1016/j.je....
 
22.
Ravichandran M, Baskaran M, Santschi PH and Bianchi TS, 1995. Geochronology of sediments in the Sabine-Neches estuary, Texas, USA. Chemical Geology 125(3–4): 291–306, DOI 10.1016/0009-2541(95)00082-W. http://dx.doi.org/10.1016/0009....
 
23.
Schelske CL, Peplow A, Brenner M and Craig N, 1994. Low-background gamma counting: applications for 210Pb dating of sediments. Journal of Paleolimnology 10(2): 115–128, DOI 10.1007/BF00682508. http://dx.doi.org/10.1007/BF00....
 
24.
Szczepańska A, Zaborska A, Maciejewska A and Kuliński K, 2012. Distribution and origin of organic matter in the Baltic Sea sediments dated with 210Pb and 137Cs. Geochronometria 39(1): 1–9, DOI 10.2478/s13386-011-0058-x. http://dx.doi.org/10.2478/s133....
 
25.
Tylmann W, 2004. Estimating recent sedimentation rates using 210Pb on the example of morphologically complex lake (Upper Lake Raduñskie, N Poland). Geochronometria 23: 21–26.
 
26.
United Nations Scientific Committee on Effects of Atomic Radiation, 2000. Exposures from Natural Radiation Sources, UNSCEAR Report, New York.
 
27.
Zaborska, A, Carroll J, Papucci C and Pempkowiak J, 2007. Intercomparison of alpha and gamma spectrometry techniques used in 210Pb geochronology. Journal of Environmental Radioactivity 93(1): 38–50, DOI 10.1016/j.jenvrad.2006.11.007. http://dx.doi.org/10.1016/j.je....
 
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